Integral Neutron Thermalization [annual summ rpt Oct 66 -

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Tank of molten diphenyl at v a r i o u s poison (ethyl b o r a t e ) concentrations. 2. Position-dependent s p e c t r u m m e a s u r e m e n t s around the i n t e r 0 f a c e between a 1 2 in. by 8 in. by 4 in. tank of molten (80 C ) diphenyl a d j a c e n t to a 1 2 in. by 8 in. by 1 2 in. tank of D 0 at 2 the s a m e t e m p e r a t u r e . The diphenyl was poisoned by ethyl b o r a t e to 3 . 197 F i g . 4. g--Definitions and l e a s t s q u a r e s values f o r a 9 p a r a m e t e r V F F f o r the out-of-plane vibrations of diphenyl.

Considerable s t r u c t u r e i n the one-phonon double d i f f e r e n t i a l s c a t t e r i n g c r o s s s e c t i o n is predicted by the new model, but the d a t a a r e not yet sufficiently p r e c i s e to provide a good t e s t of t h e s e predictions. m e n t with neutron d a t a - Nevertheless, over-all agree- both i n t e g r a l and differential - and,particularly, a g r e e m e n t with specific h e a t d a t a indicates t h a t the c e n t r a l f o r c e model r e p r e s e n t s a d i s t i n c t i m p r o v e m e n t o v e r previous phenomenological models.

The definition f o r the diphenyl molecule of t h e s e c o o r d i n a t e s is d e s c r i b e d i n ' F i g . 4. 7. ; the change i n t h e angle 1 C. bond ( X = H, o r the C in the adjacent ring) and t h e plane 1 1 m, f o r m e d b y t h e i - t h c a r b o n a t o m a n d its two a d j a c e n t c a r b o n neighbors; Ari = t h e change i n angle between Ci-lCiCi+ , C i + 2 plane. In F i g . 8 the coordinates d e s c r i b i n g the out-of-plane motions a r e specified. B e c a u s e diphenyl i s a planar molecule, i t s n o r m a l v i b r a t i o n s a r e of two kinds.

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